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 Scope and Limitations of the T-Reaction. The Tert.-amino-effect in the Synthesis of Chiral Heterocycles
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Scope and Limitations of the T-Reaction. The Tert.-amino-effect in the Synthesis of Chiral Heterocycles

издательство Книга по Требованию Физическая химия
Cтраниц 204        мягкая обложка       
Аннотация:An increasingly popular entry into tetrahydroquinolines is represented by the T-reaction, i. e. a subtype of the transformations relying on the isomerization-cyclization sequence known as the tert. -amino-effect. The latter was shown to proceed via a most remarkable helical dipolar intermediate generated upon a hydrideshift from an alpha-amino-C-H in tert. -anilines to an unsaturated ortho-substituent, accomplishing C-C-bond formation from a nonactivated NCH-moiety. The tert. -amino-effect was first brought to the attention of the synthetic community in the seminal contribution of O. Meth-Cohn and H. Suschitzky from 1972. The quinoline motif is an integral part of a wide variety of bioactive classes of compounds. Since then, the protocol has progressively evolved into a convergent, economical and yield-efficient preparation of structurally diverse, highly functionalized and pharmacologically valuable heterocycles, bearing stereoselectively introduced centers of chirality.
Издательство: Книга по Требованию
Год:2008
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Поиск: Scope and Limitations of the T-Reaction. The Tert.-amino-effect in the Synthesis of Chiral Heterocycles
НОВЫЙ ГОД СИМВОЛ 2013 ГОДАУКРАШЕНИЯ
КАРНАВАЛ НА НОВЫЙ ГОД РАСПРОДАЖА
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